Article V of the Constitution defines how the Constitution can be amended.
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Article IV of the Constitution outlines the duties states have to each other, and the duties the federal government has to the states. It provides for the admission of new states and defines a process for changing state boundaries. It also originally included the Fugitive Slave clause, which is now obsolete.
Article III of the Constitution identifies the third branch of our separated government, empowering the courts to decide cases and limiting them to the exercise of a certain kind of authority. It establishes the Supreme Court of the United States, and defines the crime of treason, the only crime listed in the Constitution.
Article I of the Constitution defines the role of Congress, the federal legislative branch. Sections 9 and 10 of Article I list which powers are denied to Congress and the States.
Article I of the Constitution defines the role of Congress, the federal legislative branch. Section 8 contains the enumerated powers of the federal government delegated to Congress.